We study the local dynamical fluctuations in glass-forming models of particles embedded in d-dimensional space, in the mean-field limit of d - ???. Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, ??2. The d - ??? local dynamics therefore becomes quite rich upon approaching the glass transition. The finite-d remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of ??2 around the glass transition that is not based on multiparticle correlations.
Local Dynamical Heterogeneity in Simple Glass Formers / Biroli, G; Charbonneau, P; Folena, G; Hu, Y; Zamponi, F. - In: PHYSICAL REVIEW LETTERS. - ISSN 0031-9007. - 128:17(2022). [10.1103/PhysRevLett.128.175501]
Local Dynamical Heterogeneity in Simple Glass Formers
Zamponi F
2022
Abstract
We study the local dynamical fluctuations in glass-forming models of particles embedded in d-dimensional space, in the mean-field limit of d - ???. Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, ??2. The d - ??? local dynamics therefore becomes quite rich upon approaching the glass transition. The finite-d remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of ??2 around the glass transition that is not based on multiparticle correlations.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.


